Simeoni received his episcopal consecration on the following April 4 from Cardinal Alessandro Franchi, with Archbishops Edward Henry Howard and Pietro Villanova Castellacci serving as co-consecrators, in the chapel of the Pontifical Urban Athenaeum of Propaganda Fide.
On 28 September 1883 he was appointed Bishop of Luxembourg, and was consecrated on 4 November of the same year by Cardinal Edward Henry Howard.
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