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Among the original songs by Nilsson, were one by Phil Spector (who had earlier co-written a song with Nilsson), Jeff Barry and Ellie Greenwich, "River Deep - Mountain High", and two by The Beatles; She's Leaving Home and "You Can't Do That", the latter in an arrangement that quoted twenty other Beatles lyrics.
The group hit the top of the charts in 1964 with "Chapel of Love," a song that Phil Spector, Jeff Barry and Ellie Greenwich had originally written for The Ronettes.