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She appeared in many Italian and French films in the 1950s and 1960s, notably in Claude Autant-Lara's film Le rouge et le noir in 1954, opposite Gérard Philipe.
Urondo also collaborated in the writing of movie scripts such as Pajarito Gómez (which includes a cameo appearance) and Noche terrible, and adapted for television Flaubert's Madame Bovary, Stendhal's Le Rouge et le Noir, and Eça de Queiroz's Os Maias.
In New York City he and his wife, Princess Norina Matchabelli (an actress whose stage name was Maria Carmi), opened a small antiques shop, Le Rouge et le Noir, at 545 Madison Avenue.