Their elder brother Sir Robert Eden, 1st Baronet, of Maryland (second son of the third Baronet of West Auckland), was the great-great-grandfather of Prime Minister Anthony Eden, 1st Earl of Avon, and the great-great-great-grandfather of the Conservative politician John Benedict Eden, Baron Eden of Winton.
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However, Governor Robert Eden disputed Harford's inheritance, and in 1774 tried to claim a part of the estate on behalf of his wife Caroline.
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On 26 April 1763 she married Maryland's last colonial governor, Robert Eden (1741–1784).
The Right Reverend Robert Eden, third son of the second Baronet of Maryland, was Primus of Scotland and Bishop of Moray, Ross and Caithness.