He was also an architect and designed many churches in the south of England such as St Francis of Assisi Church in Birmingham and Our Lady of Loreto and St Winefride's Church in London.
He promised to bear all the expenses of creating a convent, and helped by an endowment of £2000 from the Earl of Shrewsbury he commissioned Augustus Pugin to design the building for them.
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Before being ordained to the priesthood, Bishop Barbarito served as a deacon at St. Francis of Assisi Church, Astoria, Queens, for one year.