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In 1617 Sylvius accompanied Malapert on his return to the Southern Netherlands, where they both spent twelve years at the University of Douai.
In 1688, having taken the bachelor's degree at the University of Douai, he spent two months as tutor of divinity at Magdalen College, Oxford, which James II of England purposed making a seat of Catholic education.
After completing his course of humanities at Mons, he studied philosophy at the Catholic University of Leuven and theology at University of Douai, in a seminary founded by the bishop of Cambrai in connection with the faculty of theology.