Several people influential in the United States during the 19th century, including Francis Scott Key, Associate Supreme Court Justice Bushrod Washington, and U.S. Mint Director James Pollock, served as officers of the mission; many others supported the mission in other ways.
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Its Home Office in Villanova, Pennsylvania, was designed by Horace Trumbauer.
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In addition to its primary work of starting Sunday schools in rural communities, the Sunday and Adult School Union became known for its publications and its ticket reward system for Sunday school students who memorized Scripture.
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