Becoming marquis de Montausier at the death of his elder brother in 1635, he was the recognised aspirant for the hand of the Catherine de Vivonne, marquise de Rambouillet|
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She was married at the age of twelve to Charles d'Angennes, vidame du Mans, and afterwards marquis de Rambouillet.
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Occasionally, in spring and summer, the marquis and marquise de Rambouillet would entertain the habitués of their Parisian residence in the château de Rambouillet.
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In homage to the Marquise de Rambouillet, the city of Rambouillet has named its Junior High School Collège Catherine de Vivonne.