On 27 April 1861 he married the distinguished painter, Ann Mary, daughter of Joseph Severn, himself a painter and the friend of Keats, who had succeeded Newton in Rome; she died in 1866 at their residence, 74 Gower Street, Bloomsbury.
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In 1889, he was presented by his friends and pupils, under the presidency of the Earl of Carnarvon, with a testimonial in the form of a marble portrait bust of himself by Boehm, now deposited in the Mausoleum room at the British Museum ; the balance of the fund was by his own wish devoted to founding a studentship in connection with the British school at Athens.
In September 1855, Smith was gazetted to Lieutenant and in the following October was chosen to lead a small group of Royal Engineers bound to help Charles Thomas Newton's archaeological mission to the remains of the ancient civilisation at Knidos in Turkey.
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