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Starting in 1985, Mellon also worked under the direction of Philippe Herreweghe, with La Chapelle Royale (1985–1990) and the Collegium Vocale Gent (1990–1996), interpreting Charpentier, Heinrich Schütz, Monteverdi, Jean Gilles, and Johann Sebastian Bach.
The initial vocation of the ensemble was to interpret the great French repertoire of the 17th century (Henri Dumont, Jean-Baptiste Lully, Marc-Antoine Charpentier, André Campra, Jean Gilles...) but, since 1985, Herreweghe associated it more and more with his own Belgian ensemble, the Collegium Vocale Gent, in a repertoire almost exclusively dedicated to Johann Sebastian Bach.