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He expelled the Jesuits from Malta, in line with similar acts taken in his homeland Portugal and its Empire, as well as in the Two Sicilies of which Malta was a vassal, and in France, the Spanish Empire and Parma.
When Charles III of Spain ordered the expulsion of the Jesuits from all Spanish dominions in 1767, the Jesuit mission on Leyte was handed over to the Augustinians.
El Colegio del Príncipe, established by Royal Decree of King Carlos III after the expulsion of the Jesuits, was the former "college of chiefs" of the native nobility, created during the reign of Viceroy Francisco de Borja y Aragón Príncipe de Esquilache in Lima.
On October 12, 1897, he entered the noviciate of the German Province of the Society of Jesus (Jesuits), which then was located in Bleijenbeek (Netherlands) due to the expulsion of the Jesuits during the Kulturkampf of the German Reich.
With the expulsion of the Jesuits in 1759, by order of the Marquis of Pombal, the church was donated to the University of Coimbra until its purchase by the Discalced Friars of the Order of Saint Augustine that were there from 1780 to 1832.