His Portrait of Gertrude Stein (1907) was painted as an apparent response to Picasso's portrait of the previous year, and in The Autobiography of Alice B. Toklas Stein described the very methodical way in which Vallotton painted it, working from top to bottom as if lowering a curtain across the canvas.
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He is mainly remembered for the mark he left on several special issues of Paris journals, most notably l'Assiette au beurre, contributors to which included Kees van Dongen, Félix Vallotton, František Kupka, Steinlen, Adolphe Willette, and Jacques Villon.