Rayne and his wife divorced in 1960 and on 2 June 1965, he married Lady Jane Vane-Tempest-Stewart (a daughter of the 8th Marquess of Londonderry and sister of Lady Annabel Goldsmith) and they had four children: Natasha Deborah (b. 1966), Nicholas Alexander (b. 1969), Tamara Annabel (b. 1970) and Alexander Philip (b. 1973).
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