In 1911, he was a Papal Ablegatus for the imposition of the red biretta on Cardinal Enrique Almaraz y Santos, Archbishop of Seville.
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Alfrink received his episcopal consecration on the following 17 July from Archbishop Paolo Giobbe, papal internuncio in The Hague, with Bishops Willem Lemmens and Jan Smit serving as co-consecrators, in St. Catherine's Cathedral.