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The 14-track album features 12 original tracks and cover versions of Pink Floyd's "See Emily Play" and, as a bonus track in some countries, the Eurythmics' "Love Is a Stranger".
The focus of the film is Syd Barrett, the lead vocalist and guitarist of the early Pink Floyd, who created their unique psychedelic sound and most of the band's early songs, including the singles "Arnold Layne" and "See Emily Play" and much of their first album The Piper at the Gates of Dawn.
In May 2007 Martha Wainwright, her mother, Kate McGarrigle, and cousin Lily Lanken performed "Golden Hair" and "See Emily Play" at the Syd Barrett memorial concert at the Barbican Centre in London.