Sir Charles was married on 7 December 1866 to Harriet Sarah Moncreiffe (7 February 1848 – 9 May 1906), daughter of a Scottish baronet.
Sir Charles Mordaunt, 6th Baronet (1697? – 11 March 1778), of Walton d'Eiville in Warwickshire, was an English landowner and Tory Member of Parliament (MP).
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The following year he was cited as one of two co-respondents in the case for divorce brought by Sir Charles Mordaunt, 10th Bt., a former M.P., against his wife, Harriet, in which Prince Albert Edward, The Prince of Wales (later King Edward VII), was called to give evidence.
His uncle, Sir Charles Mordaunt, 10th Baronet, was involved in a sensational divorce case of 1870 that concerned, among other things, a possible relationship between his wife Harriet and the Prince of Wales.