He was born at Aberystwyth, his father being a merchant and a pioneer of Welsh Methodism, and his mother a niece of Thomas Charles of Bala.
In the 1780s Thomas Charles held the curacy of Lovington along with several other local parishes.
He had learned of Robert Raikes's Sunday Schools before he left the Establishment, but he preferred his own system.
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This was enough to make him unpopular with many of the Welsh clergy, and being denied the privilege of preaching for nothing at two churches, he helped his old Oxford friend John Mayor, now vicar of Shawbury, Shropshire, from October until 11 January 1784.
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From April 1799 to December 1801 six numbers of a Welsh magazine called Trysorfa Ysprydol (Spiritual Treasury) were edited by Thomas Jones of Mold and himself; in March 1809 the first number of the second volume appeared, and the twelfth and last in November 1813.
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In 1800, when a frostbitten thumb gave him great pain and much fear for his life, his friend, Rev. Philip Oliver of Chester, died, leaving him director and one of three trustees over his chapel at Boughton; and this added much to his anxiety.
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The Groveland Four (or the Groveland Boys) were four men, Ernest Thomas, Charles Greenlee, Samuel Shepherd and Walter Irvin, who were falsely accused of rape in Lake County, Florida, USA, in 1948.
One of his wives were Edith Mary Sowebry, daughter of Thomas Charles Johnson Sowerby and sister-in-law of Lady Mabel Annesley.
Thomas Charles Bigge (died 1794) was High Sheriff of Northumberland for 1771.
Thomas Charles "Tom" Kilbey (born 19 October 1990) is an English television star and Designer.
Cogwagee (Thomas Charles Longboat) (June 4, 1887 – January 9, 1949) was an Onondaga distance runner from the Six Nations of the Grand River First Nation Indian reserve near Brantford, Ontario, and for much of his career the dominant long distance runner of the time.