At the age of eighteen he became a pupil of Dr. Denman, the eminent London accoucheur, attending William Hunter's and Fordyce's lectures.
He also chaired the Committee of Inquiry into the Amritsar massacre which condemned the conduct of General Reginald Dyer.
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Also in 1775, Carlini was commissioned by Dr William Hunter, first Professor of Anatomy at the Royal Academy schools, to make a cast of the flayed corpse of a recently executed smuggler.