Sancroft was a patron of Henry Wharton (1664–1695), the divine and church historian, to whom on his deathbed he entrusted his manuscripts and the remains of Archbishop Laud (published in 1695).
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Practical efforts were made in the religious households of Nicholas Ferrar at Little Gidding, 1625, and of William Law at King's Cliffe, 1743; and under Charles II, says Fr. Bede in his Autobiography, “about 12 Protestant ladies of gentle birth and considerable means” founded a short-lived convent, with William Sancroft, then Dean of St Paul's, for director.
In 1688, the issue arose during the trial of the Seven Bishops—William Sancroft, Archbishop of Canterbury; Sir Jonathan Trelawny, 3rd Baronet, Bishop of Winchester; Thomas Ken, Bishop of Bath and Wells; John Lake, Bishop of Chester; William Lloyd, Bishop of Worcester; Francis Turner, Bishop of Ely and Thomas White, Bishop of Peterborough—by a common jury.
Vossius introduced him to William Sancroft, who collated him (after the revocation of the Edict of Nantes in 1685), to the rectory of Eynesford in Kent on 18 November 1687, having previously made him a librarian (perhaps assistant to Henry Wharton, recruited by Sancroft at the same period) at Lambeth Palace.