When the Ottomans crossed the Bahlui River in Iaşi on 25 June 1821, Lieutenant Catakouzenos and his forces, originally stationed on the Russian frontier, crossed the Prut River.
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He took part in the Battle of Sculeni on June 29, 1821 where Ottoman forces chased him (along with Yiannis Pharmakis and a small force of 400 Greeks) to the Secu Monastery in Neamţ county where the Greeks made their last stand.