He married Eulalie Joséphine Biju-Duval d'Algreis in 1811, and they had a child, who was portrayed by Eugène Delacroix in 1828 (the portrait is in McIlhenney Collection in Philadelphia, U.S.).
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Charles Théophile Angrand was born in Criquetot-sur-Ouville, Normandy, France, to schoolmaster Charles P. Angrand (1829–96) and his wife Marie (1833–1905).