While continuing to appear on the Opry, Copas recorded several other hits during the late 1940s and early 1950s, including "Signed Sealed and Delivered", "The Tennessee Waltz", "Tennessee Moon", "Breeze", "I'm Waltzing with Tears in My Eyes", "Candy Kisses", "Hangman's Boogie", and "The Strange Little Girl".
Country music singers Patsy Cline, "Cowboy" Lloyd Copas and Hawkshaw Hawkins were on board a Comanche owned and piloted by Cline's manager, Randy Hughes, when it crashed in deteriorating weather near Camden, Tennessee on March 5, 1963, killing all on board.
He toured with Skinner and also worked with country musicians such as Pee Wee King, Cowboy Copas, and Ray Price.
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"Signed Sealed and Delivered", a 1948 song by Cowboy Copas later covered by James Brown