In 1965 he was appointed professor of government at the new University of Kent at Canterbury, and from 1970 to 1974 he was Master of Darwin College, Kent.
In 1958, funded by the British Council, he joined the Biochemistry Department at the University of Cambridge at Darwin College to work for a PhD under Malcolm Dixon on the mechanism of metal activation of the enzyme phosphoglucomutase.
In 1964 Darwin College, Cambridge was founded with support from the Rayne Foundation and a personal donation from Rayne himself, and this is acknowledged by the college in two notable ways: Firstly, on the college's coat of arms, which superimposes Rayne's coat of arms alongside that of the Darwin family's where the college gains its namesake.
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Sir Moses I. Finley, CBE, FBA (May 20, 1912–June 23, 1986) was an American professor, whose prosecution by the McCarran Security Committee led to his move to England, where he became English classical scholar and eventually master of Darwin College, Cambridge.
Frank George Young (1908–1988), biochemist and first Master of Darwin College, Cambridge