George married December 6, 1837, the stepdaughter of his brother, Loammi Baldwin, Jr., namely, Catherine Richardson Beckford, daughter of Captain Thomas and Catherine (Williams) Beckford, of Charlestown.
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The canal served its uses until superseded by the Boston and Lowell Railroad.
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In his fourteenth year he made some sketches of the fortifications of Boston harbor in the war of 1812, of which his brother Loammi Baldwin, Jr. was the chief engineer.
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The following were some of his early engagements: 1821, built P. C. Brook's stone bridge; 1822–1823, in Pennsylvania with his brother; 1823–1825, at factories in Lowell; 1826, surveyed Charlestown Navy Yard also known as the Boston Navy Yard in Charlestown; executed Marine Railway; 1831–1833, in England; 1833–1834, on the Boston and Lowell Railroad; 1834–1836, in Nova Scotia; 1837, in Georgia, on Brunswick Canal.
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His five sons, Cyrus Baldwin (1773–1854), Benjamin Franklin Baldwin (1777–1821), Loammi Baldwin, Jr. (1780–1834), James Fowle Baldwin (1782–1862), and George Rumford Baldwin (1798–1888) were also well-known engineers.