She thus became a ward of her stepmother's relation George Campbell, 8th Duke of Argyll, growing up at his Inveraray Castle and marrying his second son Lord Archibald Campbell (1846–1913) on 12 January 1869 (their children included Niall Campbell, 10th Duke of Argyll).
In 1805 Pye was entrusted by Heath with the execution of a plate of Inveraray Castle from a drawing by J. M. W. Turner.
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