In 1813, Langeron was put in charge of the blockade of Thorn, and later that year he commanded a corps at Koenigswarte, Bautzen, Siebeneichen, Lowenberg, Katzbach, and Leipzig.
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In 1812, Langeron was given command of a corps in the Army of the Danube with which he fought at Brest-Litovsk and on the Berezina.
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After the Napoleonic wars, Langeron was appointed the Military Governor of Kherson and Odessa, the commander-in-chief of the Bug and Black Sea Cossacks, and the Governor of Yekaterinoslav, Kherson, and Crimea.
Held by French troops led by Claude Legrand and Pierre Margaron, it was attacked by two Russian columns under the command of Louis Alexandre Andrault de Langeron and I. Przebyszewski.
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He also served as a temporary Governor General of Novorossiia for nearly a year, from July 1822 to May 23, 1823, between Governors General Alexandre Langeron and Mikhail Vorontsov.