Mark Kac, Probability and related topics in the physical sciences. 1959 (with contributions by Uhlenbeck on the Boltzmann equation, Hibbs on quantum mechanics, and van der Pol on finite difference analogues of the wave and potential equations, Boulder Seminar 1957).
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The founders of the theory were Paul Erdős, Aurel Wintner and Mark Kac during the 1930s, one of the periods of investigation in analytic number theory.
Among his numerous contributions, the most famous one is a general construction of isospectral manifolds (1985), which is based on his geometric model of number theory, and is considered to be a breakthrough in the problem proposed by Mark Kac in "Can one hear the shape of a drum?" (see Hearing the shape of a drum).