During the war, she went to Rouen in the spring of 1915, helping to run the canteen at the railhead there for four weeks, then returning to help her father at the Oxford University Press, but finally returning to France in the espionage department at the War Office Department in Paris (1918), where she was finally reunited with her fiancé Bevil Quiller-Couch.
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Pope is prominently remembered first for her pro-war poetry, but also as a representative of homefront female propagandists such as Mrs Humphry Ward, May Wedderburn Cannan, Emma Orczy, and entertainers such as Vesta Tilley.