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He was sent to Carlow College as a lay student, and in 1816 entered Maynooth, where he became proficient in natural philosophy and languages.
In 1992, he became lecturer in mathematical physics at Maynooth College, The National University of Ireland, subsequently was Royal Society postdoctoral fellow at the University of Innsbruck, Austria, lecturer in Mathematical Sciences Department at the University of Durham, UK, and held a postdoctoral position at La Sapienza University in Rome, Italy.
He was also professor of medicine in the Roman Catholic university medical school, a senator of the Royal University of Ireland, 1880, crown nominee for Ireland in the General Medical Council of the United Kingdom on 29 November 1881, physician to the House of Industry hospitals, and visiting physician to Maynooth College.
He was educated at Carlow College as a lay student from 1885 to 1889, and went to Maynooth College to Study for the priesthood, where he was invited to write an ode on the college's centenary; however, he left priestly formation due to ill health.
MacRory taught Scripture and Modern Theology at St Mary's College, Oscott in England until 1889, when he was appointed Professor of Scripture and Oriental Languages at his alma mater of Maynooth College.