In addition to his screen work, Mercurio remains active in the theatre, most notably as a member of The Actors' Gang theatre in Los Angeles, which was founded by acclaimed actor Tim Robbins.
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When he was a teenager, they relocated to Ridgewood, New Jersey, where Mercurio attended Ridgewood High School from 1986 until 1988.
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In 2010, Mercurio played a disenchanted former soldier who has been recruited to build a bomb for a domestic terrorist, in the independent suspense-thriller Elevator, written and produced by Marc Rosenberg (Dingo, December Boys) and directed by Stig Svendsen (The Radio Pirates).
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