Many of the species found on the mountain are unique to the Comoros and four bird species are found only on the slopes of Mount Karthala: Humblot's Flycatcher, Comoro White-eye, Comoro Drongo and Karthala Scops Owl.
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Pheidole vulcan is known only from the slopes of the two volcanoes Mt. Karthala and La Grille, at elevations between 995 and 1125 m on Grande Comore and thus is possibly an endemic species of the island.