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Initially tutored by his father, he went to the Royal Academy Schools early in 1808, but in the same year, after a disagreement about his art studies, ran away to sea as a Midshipman in the Royal Navy.
On 25th August 1794 he was apprenticed to Benjamin Smith for seven years and ultimately trained in engraving techniques at the Royal Academy Schools under Francesco Bartolozzi.
He trained at King's College London and University College, London, and joined his father's practice in 1884, also studying at the Royal Academy Schools, the Architectural Association, and the École des Beaux-Arts, Paris.
Also in 1775, Carlini was commissioned by Dr William Hunter, first Professor of Anatomy at the Royal Academy schools, to make a cast of the flayed corpse of a recently executed smuggler.