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However, Solana would be most known for his spell at Real Zaragoza, where he would add one Spanish Cup to his cabinet as well as the memorable 1994–95 UEFA Cup Winners' Cup against Arsenal, appearing in more than 300 overall official matches for the Aragonese.
He was seriously injured in his first season, but bounced to back to be an important first-team element in the conquest of two leagues and one Spanish Cup, being fairly used even after the 1994 purchase of Fernando Redondo.
In mid-November 2008, Sergio signed with CA Osasuna until the end of the top flight season, as the Navarrese lost Rovérsio for its duration due to a serious knee injury in a Spanish Cup contest against Getafe CF.
In 1985, he returned to New York and subsequently became the 1987 Champion of the Mayor's Cup in Washington, DC, the Spanish Cup and the New York State Golden Gloves.