In September 2008, The CW announced Holland would appear in three episodes of the second season of the teen-drama television series Gossip Girl, created by The O.C. creator Josh Schwartz.
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She also made a notable cameo appearance in the film The Last Song, and she played the teen-temptress role of Janice Heddon in the film Straw Dogs, a remake of the 1971 film of the same name.
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