From 1849 to 1853, Crummell studied at Queens' College, Cambridge, sponsored by Benjamin Brodie, William Wilberforce, Arthur Penrhyn Stanley, James Anthony Froude, and Thomas Babington Macaulay.
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He wrote the poem "Freedom," which celebrated the British abolitionist Thomas Clarkson; it was published in Alexander Crummell's 1849 biography of Clarkson.