The Tondo Province annexed to this new district the towns of Cainta, Taytay, Antipolo and Boso-boso, while Laguna contributed the towns of Angono, Binangonan, Cardona, Morong, Baras, Tanay, Pililla and Jalajala.
This consisted of the towns of Antipolo, Bosoboso, Cainta and Taytay from the Province of Tondo; and the towns of Morong, Baras, Tanay, Pililla, Angono, Binangonan and Jalajala from the Province of La Laguna, with the capital at Morong.
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Antipolo, Taytay and Cainta serve as the economic centers of the province, while Angono, Rodriguez, Morong, San Mateo, Tanay, Binangonan and Teresa are taking successful steps to urbanize areas within their jurisdiction.
The diocese extended over the provinces of Camarines and Albay as far as and including the islands of Ticao, Masbate, Burias and Catanduanes; the province of Tayabas as far as and including Lucban; and, in the contracosta of Mauban to Binangonan, Polo, Baler and Casiguran.
In 1992, a public school in Binangonan, Rizal was built and was named after him, the Vicente Madrigal Municipal High School.