His first studio album through his new record label, Unveil, was released on May 22, 2007.
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In January 2010, Jeff joined the music department of North Central University in Minneapolis, MN as a faculty member.
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The song "More Love, More Power" can be added to the Christian video game Dance Praise song list via the Dance Praise Expansion Pack Volume 3: Pop & Rock Hits.
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The Worship Collection (June 19, 2007) Greatest hits album
Jeff Beck | Jeff Koons | Jeff Foxworthy | Jeff Buckley | Jerry Jeff Walker | Jeff Daniels | Jeff Bezos | Jeff Minter | Jeff Tweedy | Jeff Sagarin | Jeff Bingaman | Jeff Goldblum | Jeff Bridges | Jeff Porcaro | Jeff Hardy | Jeff Bennett | Jeff Wall | Jeff Kennett | Jeff Gordon | Jeff Jarrett | Jeff Garlin | Jeff Flake | Jeff Fisher | Jeff Coffin | DJ Jazzy Jeff | Jeff Stelling | Jeff Martin | Jeff Wayne's Musical Version of The War of the Worlds | Jeff Rowley | Jeff Probyn |
The reviewer for Crosswalk gave the album a B, noting that MercyMe reminded him of "SONICFLOOd before Jeff Deyo's departure" and describing lead singer Bart Millard's vocals as "raw, somewhat scratchy, and unique", while criticizing the overall consistency of the songs record.