The original building dates to the thirteenth century when it was owned by the MacSweens.
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In the 2010 Channel 4 programme Dom Joly and the Black Island, Joly and Tintinologist Michael Farr identify Castlebay and Kisimul as the locations of Kiltoch and the Ben More Castle used as settings in The Adventures of Tintin comic The Black Island, although the scenes of reaching it by boat and exploring it on foot were filmed at Lochranza Castle on the Isle of Arran.