Under the Carolingian dynasty Bondo belonged to the Ministerium Bergallia, which was a dependant of the early Bishops of Chur, though after 960 it was owned directly by the Bishop.
The diocese include nine orders of men and ten orders of women (Franciscans, Augustinians, Dominicans, Benedictines, and others), as well as eleven congregations.
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These two missions, Rhætiæ and Mesauci, were made prefectures Apostolic under the care of Italian Capuchins and these prefects resided in the towns of Obervaz and Cama, both in the Canton of Graubünden.
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Three Benedictine abbeys — Einsiedeln, Engelberg, and Disentis — are within the diocese and, with the church of Saint Nicholas of Flüe at Sachseln, are places of pilgrimage.
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Already in use by the Romans, during the Middle Ages the Septimer Pass was crucial to the temporal power of the Bishopric of Chur whose extensive territories until the fourteenth century included Chiavenna.