After becoming acquainted with Joseph Pignatelli and following Pope Pius VII's restoration of the Society of Jesus, he planned on entering the Society but failed due to the resistance of his sister Vittoria, who desperately sought to live near her brother.
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Odescalchi died without a direct heir in 1713, and his titles and fortune were inherited by his relative Baldassare Erba-Odescalchi (1683-1746), the grandson of Alessandro Erba (1599-1670) and Lucrezia Odescalchi, the sister of Innocent XI and Carlo Odescalchi.
Livio Odescalchi was born in Rome in 1655, the son of Carlo Odescalchi (1607-1673) and Beatrice Cusani.